Amount and characteristics of microplastic and organic matter in wind-blown sediment at different heights within the aeolian sand saltation layer.

Soils of croplands especially where plastic film mulch is commonly applied, are normally contaminated by Microplastics (MPs). Microplastics can threaten air quality, food and water health, as well as human health by wind erosion processes. In this research, we investigated MPs collected in four wind erosion events at sampling heights between 0 and 60 cm in typical semiarid farmlands in northern China that employ plastic film mulch. Height distribution and enrichment heights of the MPs were measured. The results revealed that the average amounts of MPs for 0-20 cm, 20-40 cm and 40-60 cm sampling heights were 868.71 ± 249.21, 799.87 ± 271.25, 1102.54 ± 317.44 particles kg-1. The average enrichment ratios of MPs for the different heights were 0.89 ± 0.54, 0.85 ± 0.56, 1.15 ± 0.73. Height distribution of MPs was combined affected by shape (fiber and non-fiber) and size of MPs, wind speed and soil aggregate stability. The amount of fibers approximately <4 mm in size and non-fibers <2 mm in size increased with sampling height, while both shapes of larger MPs than these two sizes was almost independent of the sampling height. Enrichment ratios of microfibers were positively related to wind speed but negatively related to soil aggregate stability at each sampling height. The results revealed that although MPs have similar density to organic matter (OM), the MPs' amount and enrichment were independent of height but the OM content and enrichment ratios increased with height. These results suggested that more attention should be paid to the exploration of the influence of higher sampling heights (>60 cm) on the distribution of MPs in the future and the MPs characteristics for different sampling heights require carefully parameterization in detailed models of atmospheric MPs transport by wind erosion.

Wind erosion induced low-density microplastics migration at landscape scale in a semi-arid region of northern China.

Microplastics (MPs) have been extensively investigated in terrestrial environments, while the occurrence and movement of MPs at the landscape scale in semi-arid regions with serious wind erosion are less well studied. Here, we sampled film mulching farmland and downwind nearby grassland surface soils in a semi-arid region of northern China to explore the distribution of MPs at different downwind distances and the potential environmental risk to the local landscapes. The results revealed that the MP abundances presented a decreasing trend with increasing downwind distance (Mann-Kendall test, P < 0.01). The MP size distributions at different distances showed similar sigmoid trends described by logistic models. MP fiber size (500-2000 µm) abundance in the farmland was higher than that of the grassland. By contrast, MP non-fiber size (<1000 µm) abundance of farmlands was less than that of the grassland. The abundances of fibers larger than 500 µm and non-fibers larger than 1000 µm in size decreased exponentially with increasing downwind distance. The size of transported MPs at the landscape scale was larger than that of long-distance dispersal. The migration of MPs from farmlands can pose a potential threat to the downwind landscape, leading the downwind grassland to be a potential MP emission source. This study presents the first insights into the MPs distribution among different downwind distances at the landscape scale. Future research is required to deploy aeolian sediment sampling devices and establish the connection between the field data and the MP emission models.

Plastic mulch film induced soil microplastic enrichment and its impact on wind-blown sand and dust.

Microplastics (MPs) pollution is being increasingly recognized as a global concern in all environments. Wind-blown sand and dust contaminated by MPs are an important pathway of MPs transport across different environments, which can result in on-site and off-site potential MP pollution. Here, we designed field experiments to detect MPs in surface soil and wind-blown sand and dust in farmlands with and without film mulch in a semi-arid region of northern China. This study provides the first insights into MPs enrichment in wind-blown sand and dust deposited by natural storms. The results reveal that fibers, fragments, and films constitute the major types of MPs in farmland soil and wind-blown sand and dust. The MPs abundances of 1-3 mm, <1 mm, and 3-5 mm items kg-1 successively decrease. The enrichment of MPs in wind-blown dust is one to two orders of magnitude higher than that in wind-blown sand. For the farmlands with (without) film mulch, the MPs enrichment ratios ranged from 0.22 (0.29) to 1.35 (2.26) in the wind-blown sand and that varied from 1.79 (1.01) to 16.6 (25.79) in the wind-blown dust. Fibers are preferentially transported by wind erosion compared to fragments and films. Soil aggregating processes, wind speed, and MPs shape may influence enrichment in wind-blown sand and dust. Film mulch debris and the application of manure may be the primary sources of MPs in farmland soils. This study further highlights the importance of the transport of airborne MPs from surface soil into the atmosphere. Future research is required to establish the quantitative relationships between the MPs shape, wind speed, and surface soil properties and the MPs enrichment in wind-blown sand and dust.